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Walk straight up to her with a smile, and pull out one of her headphones.
OR if you have the balls, put it in your ear and say "I like this song"...
I hate this idea to be honest. Touching a girl or her possessions before she's even acknowledged your presence is super high on the creepy scale. An easy was to freak out a timid girl. I think smiling and motioning for her to pull out the ear phone or just talking to her until she pulls one out is a good option.
Haha, I like the directness but I have to agree unless you can really give off an open, warm, i'm not a creeper vibe, getting touchy can be highly suspect.
Smile, pantomime something like pointing to your ear while moving your lips and if shes open she'll take'em out. I find people typically listen to music in public to not be bored so once you open and cause some interesting havoc in her life she'll forget all about it.
I can remember one instance I just sat down next to a chick, pointed my body at an open angle to her and tapped her shoulder. Really didn't matter what I said as long as the body language and segway to talking to her was creepy or predator like.
The mouthing something silently, like your yelling idea from RockstarPUA is good. Pretend like your yelling and show some character and distinguish yourself from every other guy who would just tap on her shoulder.